Anyway here I go:
to build any audio system we must to start with the best audio components/items we can afford at both system chain link extremes: front end and speaker/room.
In between those system chain link extremes yours looks pretty decent/good.
Where can I start to up date your system?. Very simple: where the sound comes at your listening position ears: speakers.
NO. I’m not talking to change those Thiels, as a fact I loved Thiel speakers and had great opportunities to liste it for long periods of time even at my place with diferent models: 7, 5, 3.5, 1.2 and the 3.6 you own.
Well the 3.6 ( as any other speaker ) is far away to be " perfect " but the 3.6 has a severe problem and is a true limitation for that " more, more " you are asking for.
Problem is that so high crossover frequency between the woofer and midrange drivers: 500 hz that grows up in frequency due the JT preference for first order ( 6 db. ) crossover filters that permit that those woofers handle frequencies as high ( we can hear because those first order filters. ) as 700hz-800hz and this means really high THD levels on what you are listening.
Here you can read what I’m talking about ( read it carefully. ):
https://forum.audiogon.com/discussions/do-you-think-you-need-a-subwoofer/post?postid=310058#310058
when you liberate the 3.6 woofers of those long excursions from 100hz and down the improvement ( sure, true and real. ) in quality level of the sound you will be listening has no paragon: just fabolous, just a new improved audio system that you can’t even imagine you " have it ". Your system could be ( then. ) outperforms systems in the 300K dollars!. Believe it or not.
@m-db sugested that and ( independent of his reasons to posted it. ) he is spot on.
There are other areas where you system can be upgraded but those are latter and when you already integrated a pair of active/self powered in true stereo fashion in your today system.
Many alternatives for subwoofers but the true home system experts comes from Velodyne and for very good reasons: DD-15 or HGS-15 models can do it over any other " glamorous " subs in the market.
Btw, why do you think that the today bets quality level performance spekaers comes with dedicated active subwoofers?. Here you can see a " dream audiophile system " where those speakers comes with active subs:
https://systems.audiogon.com/systems/615
but not only those speakers but for example the top Vandersteen and many more.
Regards and enjoy the music.
R.