Just to update: talked with a number of audio room advisors who offer consulting services.
Most are just pushing their particular products.
One, in particular, who I'll call "Dennis" was particularly abhorrent example of the acoustic field. He may or may not know his stuff (probably is extremely smart), but he was talking fast, pushing hard, and coming to conclusions to sell his product clearly based on simple computer room analysis and not taking into account the odd nature of the walls and actual measurements.
Specifically, because we are deep underground, the "drywall" is not drywall, but a product designed to allow water to pass through, made with little beads and glued together (in the unlikely event of a water event).
Underneath that is six inches of a dense expanding foam. Basically, the top sheet is very close to being acoustically transparent. Not sure what is going on, but from multiple measurements with several different tools now, the walls do not really reflect much (nor produce their own sound) but are mildly absorbent of very low frequency sounds.
Long way of saying, computer room analysis is a great tool, but no substitute for direct measurements.
With that in mind, after talking with the rare consultant who actually listened to measurements, I've decided to go with about 20% bass absorption and 20% dispersion. Mounted 4" combined bass traps/dispersion immediately behind the speakers/subs (about 1.5 inches from the wall). (The gap increases the depth of sound absorbed, while decreasing the effect on higher frequencies.) This made an immediate improvement.
Going to do about 108 sf of combine bass trap and dispersion on the back wall, and a fair bit on the ceiling, depending on results of back wall.
Nothing but a simple thin carpet on the floor. My problems are low frequencies, and it would take building a pit to have something thick enough. (A carpet with pad will just absorb high/mid frequencies.) If I need more, I'll double up on the ceiling.
The only other covering I'm doing is on two metal blast doors (on the far right) that have a huge tendency to vibrate with bass and give a solid echo. Not a fan of acoustic curtains, since like carpet, they mainly just absorb higher frequencies. I've decided to use three layers of curtains -- one a heavy acoustic curtain, one that is pretty and acoustically transparent ---- AND HIDDEN IN THE MIDDLE GODAWFUL BEADS AND COINS.
Why the faux "gypsy" (er, Romani? If I was Romani, I wouldn't claim it. It's from Spencers.) -looking garbage? Dispersion. I bought twice as much as needed, and they will hang all "bunched up" and hard, facing random directions, thereby taming down that 10'x7' metal reflector of a blast door. Even better would be to have hanging wood slats, but I couldn't seem to find any. Will see what happens. Cost total of the awful beads and "coins" = $39. If that doesn't work, I have enough space in the door frame (also a giant slab of steel) to mount 6" base traps directly to the doors.