FWIW, the big advantage to passive bi-amping is being able to match amplifiers to speaker requirements. In other words, you can run a big honking amp to power your power hungry woofers to bring out their capabilities and use an amp that you love for it's midrange and high frequencies to power the mids and tweets.
If you vertically bi-amp you are using identical amplifiers on both highs and lows (oftimes a stereo amp). This can work well if you are somewhat compromised in power requirements in the first place. It also allows for short speaker cable runs and maybe more convenient placing of the amplifiers.
In your case, I wouldn't use a second pair of 601s for the mids and highs because your speakers are efficient and you would only be using a fraction of their power. A much smaller amplifier would work just fine and possibly be much less $ than a second pair of 601s.
The biggest issue when using different amplifiers for the highs and lows is matching the outputs. In my case I had to tame down the bass to match the highs, by using an attenuator between the preamp and the monoblocks.
As always, YMMV.
Bill